Synthesen trans-A2B2-substituierter Porphyrinlinker zur Darstellung photoaktiver oberflachenverankerter MOF-Dunnschichten

By (author) Stefan Marschner

Book cover: Synthesen trans-A2B2-substituierter Porphyrinlinker zur Darstellung photoaktiver oberflachenverankerter MOF-Dunnschichten

Extent: 235, 235 pages

Publisher: Logos Verlag Berlin

Subjects: Earth & Life Sciences 

Series: Beiträge zur organischen Synthese

Series volume number: 90

Language: German

Paperback (Published)

(July 2020)

ISBN: 9783832551124

5.71 x 8.27 inches

Price: $78.00

Out of stock

In der Entwicklung organischer Solarzellen hat sich die Stoffklasse der Porphyrine, unter anderem aufgrund ihrer ausgezeichneten Lichtabsorption, besonders hervorgehoben. Zudem ermoglicht eine systematisch geschichtete Anordnung der Molekule einen effizienten Energietransfer, der beispielsweise auch im Prozess der Photosynthese eine tragende Rolle spielt. Diese Dissertation leistet einen Beitrag zur Entwicklung neuer Moglichkeiten einer effektiven Umwandlung von Solarenergie durch die Verwendung oberflachenverankerter Dunnschichten metallorganischer Geruste (SURMOFs). Im Fokus steht dabei die modulare Synthese organischer, linearer A2B2-Porphyrinlinker mit metallbindenden Carboxylat-Termini, welche zur Darstellung photoaktiver SURMOFs verwendet werden. Es wurden Moglichkeiten zur Variation solcher Porphyrinlinker untersucht, wobei unter anderem eine Molekulbibliothek auf Basis eines Porphyrin-Grundkorpers erstellt wurde. Insbesondere wurden weiterhin Syntheserouten zur Verlangerung der Linker entwickelt sowie Strategien zur Ausrichtungskontrolle der Porphyrineinheiten in resultierenden Gerustverbindungen untersucht. Die synthetisierten Linker, sowie daraus erhaltene SURMOF-Strukturen wurden zudem auf ihre jeweiligen Absorptionsverhalten untersucht und Zusammenhange analysiert.

  • By (author) Stefan Marschner

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