Synthese von Kupfer(I)- und Silber(I)-Komplexen zur Untersuchung kooperativer Effekte und Anwendung in OLEDs

By (author) Jasmin Busch

Extent: 480, 480 pages

Publisher: Logos Verlag Berlin

Subjects: Earth & Life Sciences , Technical Sciences: Computer Science, Engineering, IT, & Math

Series: Beiträge zur organischen Synthese

Series volume number: 93

Language: German

Paperback (Published)

(December 2020)

ISBN: 9783832551766

5.71 x 8.27 inches

Price: $112.00

Out of stock

Synopsis
Contributing Authors

In der Mehrheit der heutigen Smartphone-Displays und in einer Vielzahl der TV-Bildschirme sind organische Leuchtdioden (kurz OLEDs) verbaut. Bei OLEDs handelt es sich um Flachenstrahler, die aus mehreren Schichten aufgebaut sind und in denen elektrochemisch Licht erzeugt wird. Die Effizienz der OLEDs hangt, neben der Kombination der einzelnen Schichten, von den in der emissiven Schicht verwendeten Emittermaterialien ab. Aktuell sind besonders Verbindungen gefragt, die thermisch aktivierte verzogerte Fluoreszenz (TADF) aufweisen. Im Vergleich zu herkommlichen Emittermaterialien, haben TADF-Emitter kurze Emissionsabklingzeiten bei gleichzeitig hohen Photolumineszenzquantenausbeuten von bis zu 100 %. Kupfer-Komplexe sind hierbei, aufgrund des grossen Vorkommens des Metalls und vergleichsweise geringer Kosten interessante Kandidaten fur OLED-Anwendungen. In dieser Arbeit wurden Emittermaterialien basierend auf Kupfer(I) weiterentwickelt und neue Emittersysteme gefunden. Dinukleare homo- und heterometallische Kupfer(I)- und Silber(I)-Komplexe wurden dargestellt, um experimentell und theoretisch die Wechselwirkungen zwischen den Metallhalogenid-Zentren der Komplexe, die auch als Kooperativitat bezeichnet wird, bestimmen zu konnen. Kooperative Effekte in mehrkernigen Komplexen spielen eine zentrale Rolle in Bezug auf deren Lumineszenz. Die untersuchten Emittermaterialien wurden weiterhin auf tetranukleare Kupfer(I)-Komplexe ausgeweitet. Ausgewahlte dinukleare Kupfer(I)-Komplexe wurden in OLEDs verbaut und damit hohe Leuchtdichten bei gleichzeitig hohen Stromausbeuten erzielt.

By (author) Jasmin Busch

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Synthese von Kupfer(I)- und Silber(I)-Komplexen zur Untersuchung kooperativer Effekte und Anwendung in OLEDs

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